# The Bloch point in uniaxial ferromagnets as a quantum mechanical object

- Andriy Borisovich Shevchenko
^{1}and - Maksym Yurjevich Barabash
^{2}Email author

**9**:132

**DOI: **10.1186/1556-276X-9-132

© Shevchenko and Barabash; licensee Springer. 2014

**Received: **4 December 2013

**Accepted: **28 February 2014

**Published: **19 March 2014

## Abstract

Quantum effects such as tunneling through pinning barrier of the Bloch Point and over-barrier reflection from the defect potential of one have been investigated in ferromagnets with uniaxial strong magnetic anisotropy. It is found that these phenomena can be appeared only in subhelium temperature range.

### Keywords

Quantum tunneling The bloch point Domain walls Vertical bloch lines uniaxial magnetic film Quantum depinning Magnetic field Potential barrier Ferromagnetic materials## Background

Mesoscopic magnetic systems in ferromagnets with a uniaxial magnetic anisotropy are nowadays the subject of considerable attention both theoretically and experimentally. Among these systems are distinguished, especially domain walls (DWs) and elements of its internal structure - vertical Bloch lines (BLs; boundaries between domain wall areas with an antiparallel orientation of magnetization) and Bloch points (BPs; intersection point of two BL parts) [1]. The vertical Bloch lines and BPs are stable nanoformation with characteristic size of approximately 10^{2} nm and considered as an elemental base for magnetoelectronic and solid-state data-storage devices on the magnetic base with high performance (mechanical stability, radiation resistance, non-volatility) [2]. The magnetic structures similar to BLs and BPs are also present in nanostripes and cylindrical nanowires [3–6], which are perspective materials for spintronics.

It is necessary to note that mathematically, the DW and its structural elements are described as solitons, which have topological features. One of such features is a topological charge which characterized a direction of magnetization vector $\overrightarrow{\mathit{M}}$ reversal in the center of magnetic structure. Due to its origin, the topological charges of the DW, BL, and BP are degenerated. Meanwhile, in the low temperature range (*T* < 1 K), $\overrightarrow{\mathit{M}}$ vector reversal direction degeneration can be lifted by a subbarier quantum tunneling. Quantum magnetic fluctuations of such type in DWs of various ferro- and antiferromagnetic materials were considered in [7–11]. The quantum tunneling between states with different topological charges of BLs in an ultrathin magnetic film has been investigated in [12].

Note that in the subhelium temperature range, the DWs and BLs are mechanically quantum tunneling through the pining barriers formed by defects. Such a problem for the case of DW and BL in a uniaxial magnetic film with strong magnetic anisotropy has been investigated in [13] and [14], respectively. Quantum depinning of the DW in a weak ferromagnet was investigated in article [15]. At the same time, the BPs related to the nucleation [16–18] definitely indicates the presence of quantum properties in this element of the DW internal structure, too. The investigation of the abovementioned problem for the BP in the DW of ferromagnets with material quality factor (the ratio between the magnetic anisotropy energy and magnetostatic one) *Q* > > 1 is the aim of the present work. We shall study quantum tunneling of the BP through defect and over-barrier reflection of the BP from the defect potential. The conditions for realization of these effects will be established, too.

## Methods

### Quantum tunneling of the Bloch point

*r*≤ Λ, where Δ is the DW width, $\mathit{r}=\sqrt{{\mathit{x}}^{2}+{\mathit{z}}^{2}}$ , $\mathit{\Lambda}=\mathit{\Delta}\sqrt{\mathit{Q}}$ is the characteristic size of BL, the Bloch point deforms a magnetic structure of BL, as is described by the following ‘vortex solutions’ [19].

where *ϕ* = arc*tg M*_{
y
}/*M*_{
x
} are the components of the vector $\overrightarrow{\mathit{M}}$. In this case, a distribution of the magnetization along the axis OY has the Bloch form: sin*θ* = *ch*^{−1}(*y*/Δ), where *θ* is the polar angle in the chosen coordinate system.

It is noted that it is the area which mainly contributes to *m*_{BP} = Δ/*γ*^{2} (*γ* is the gyromagnetic ratio) - the effective mass of BP [19]. It is natural to assume that the abovementioned region of the DW is an actual area of BP.

*ϕ*=

*ϕ*(

*z*−

*z*

_{0},

*x*),

*z*

_{0}is the coordinate of the BP's center), we can write after a series of transformations the energy of interaction of the Bloch point

*W*

_{ H }with the external magnetic field ${\overrightarrow{\mathit{H}}}_{\mathit{y}}=-\mathit{H}{\overrightarrow{\mathit{e}}}_{\mathit{y}}$ as follows:

where *M*_{
S
} is the saturation magnetization.

*H*and effective field of defect

*H*

_{ d }, we will use the Lagrangian formalism. In this case, using Equation 2 and the ‘potential energy’ in the Lagrangian function $\mathrm{L}={\mathit{m}}_{\mathrm{\text{BP}}}\frac{{\dot{\mathit{z}}}^{2}}{2}\phantom{\rule{1em}{0ex}}-\phantom{\rule{1em}{0ex}}\mathit{W}\left({\mathit{z}}_{0}\right)$, we can write it in such form

*H*

_{ d }(

*z*

_{0}) in series in the vicinity of the defect position, its field can be presented in the following form:

where *H*_{
c
} is the coercive force of a defect, *d* is the coordinate of its center, ${\mathit{D}}^{-2}={\left(\right)}_{\frac{1}{{\mathit{H}}_{\mathit{c}}}\frac{{\partial}^{2}{\mathit{H}}_{\mathit{d}}}{\partial {\mathit{z}}_{0}^{2}}}{\mathit{z}}_{0}=\mathit{d}$, *D* is the barrier width.

It is reasonable to assume that the typical change of defect field is determined by a dimensional factor of given inhomogeneity. It is clear that in our case, ${\partial}^{2}{\mathit{H}}_{\mathit{d}}/\partial {\mathit{z}}_{0}^{2}~{\mathit{H}}_{\mathit{c}}/{\mathrm{\Lambda}}^{2}$ and hence *D* ~ Λ. Note also that the abovementioned point of view about defect field correlates with the results of work [20], which indicate the dependence of coercive force of a defect on the characteristic size of the DW, vertical BL, or BP.

*z*

_{0}= 0, the ‘potential energy’

*W*has a local metastable minimum (see Figure 1), we obtain the following expression:

*ϵ*= 1 −

*H*/

*H*

_{ c }< < 1 (we are considering the magnetic field values

*H*close

*H*

_{ c }, that decreases significantly the height of the potential barrier). In addition, potential

*W*(

*z*

_{0}) satisfies the normalization condition

*z*

_{0,1}= 0 and ${\mathit{z}}_{0,2}=3\mathrm{\Lambda}\sqrt{2\mathit{\u03f5}}$ are the barrier coordinates.

It should be mentioned that Equation 5 corresponds to the model potential proposed in articles [13–15] for the investigation of a tunneling of DW and vertical BL through the defect.

*P*of the Bloch point by the formula

where $\mathit{B}=\frac{2}{\mathit{\hslash}}{\displaystyle \underset{{\mathit{z}}_{0,1}}{\overset{{\mathit{z}}_{0,2}}{\int}}\left|\dot{\mathit{z}}{\mathit{m}}_{\mathrm{\text{BP}}}\right|}\mathit{dz}$ and *ℏ* is the Planck constant.

*z*

_{0}= 0, ${\dot{\mathit{z}}}_{0}\to 0,$ and

*t*→ −

*∞*, which corresponds to the pinning of the BP on a defect in the absence of the external magnetic field, we will find the momentum of the BP and, hence, the tunneling exponent

where *h*_{
c
} = *H*_{
c
}/8*M*_{
S
}, *ω*_{
M
} = 4*πγM*_{
S
}.

*T*

_{ c }at which the quantum regime of the BP motion takes place can be derived from relations (5) and (7), taking into account the relation $\mathit{T}{}_{\mathit{c}}\phantom{\rule{0.1em}{0ex}}=\phantom{\rule{0.5em}{0ex}}{\mathit{W}}_{\text{max}}/{\mathit{k}}_{\mathit{B}}\mathit{B}$, where

*W*

_{max}is the maximal value of the potential barrier,

*k*

_{ B }is the Boltzmann constant. Thus, in accordance with the above arguments, we obtain

Substituting into the expressions (7) and (8), the numerical parameters corresponding to uniaxial ferromagnets: *Q* ~ 5–10, Δ ~ 10^{−6} cm, 4*πM*_{
S
} ~ (10^{2} − 10^{3}) Gs, *H*_{
c
} ~ (10 − 10^{2}) Oe [19] (see also articles [20, 21], in which the dynamic properties of BP in yttrium-iron garnet were investigated), *γ* ~ 10^{7} Oe^{−1} s^{−1}, for *ϵ* ~ 10^{−4} − 10^{−2}, we obtain *B* ≈ 1–30 and *T*_{
c
} ~ (10^{−3} − 10^{−2}) К.

The value obtained by our estimate *B* ≤ 30 agrees with corresponding values of the tunneling exponent for magnetic nanostructures [22], which indicate the possibility of realization of this quantum effect. In this case, as can be seen from the determination of the BP effective mass, in contrast to the tunneling of the DW and vertical BL through a defect, the process of the BP tunneling is performed via the ‘transfer’ of its total effective mass through the potential barrier.

*z*

_{in}and the instanton frequency of the Bloch point

*ω*

_{in}(see review [23]), which characterize its motion within the space with an ‘imaginary’ time

*τ*=

*it*: from the point

*z*

_{0,1}= 0 at

*τ*= −

*∞*to the point ${\mathit{z}}_{0,2}=3\mathit{\Lambda}\sqrt{2\mathit{\u03f5}}$ at

*τ*= 0 and back to the point

*z*

_{0,1}at

*τ*=

*∞*

where *p* is momentum, *m* is the quasiparticle mass, and *F* is the force acting on it.

*p*=

*m*

_{BP}

*ω*

_{in}

*ξ*, $\mathit{\xi}~\mathrm{\Lambda}\sqrt{2\mathit{\u03f5}}$. Then, taking into account Equation 9, we will rewrite Equation 10 in the following way:

Setting the abovementioned parameters of the ferromagnets and defect into Equation 11, it is easy to verify that this relationship is satisfied, that in turn indicates the appropriateness of use of the WKB approximation in the problem under consideration.

*F*, acting on the quasiparticle, with the braking force $\tilde{\mathit{F}}$,which in our case is approximately $\mathit{\alpha}{\mathit{\omega}}_{\mathit{M}}{\mathit{\omega}}_{\mathrm{in}}\mathrm{\Lambda}\sqrt{2\mathit{\u03f5}}{\mathit{m}}_{\mathrm{\text{BP}}}$, where

*α*~ 10

^{−3}− 10

^{−2}is the magnetization decay parameter. Taking into account the explicit form of

*F*, we obtain

The analysis of this expression shows that $\tilde{\mathit{F}}/\mathit{F}<<1$ at 10^{−2} ≤ *h*_{
c
} ≤ 10^{−1}, *ϵ* ~ 10^{−4} − 10^{−2} and *α* ~ 10^{−3} − 10^{−2}. The obtained result indicates that at the consideration of the BP quantum tunneling process, the effect of breaking force can be neglected.

Note also that the mechanism of breaking force has been investigated in the work [25] and is associated with the inclusion of relaxation terms of exchange origin in the Landau-Lifshiz equation for magnetization of a ferromagnet [26].

## Results and discussion

### The over-barrier reflection of the Bloch point

In the above, it was mentioned that tunneling of DW and vertical BL is carried out via sub-barrier transition of small parts of the area of DW or the length in case BL. In this case, both DW and vertical BL are located in front of a potential barrier at a metastable minimum that makes possible the process of their tunneling. At the same time, the BP depinning occurs via ‘transmission’ through the potential barrier instantly of entire effective mass of the quasiparticle. This result indicates that the presence of a metastable minimum in the interaction potential of BP with a defect (in contrast to DW or BL) is not necessary. Moreover, it means that there exists a possibility of realization for BP of such quantum effect as over-barrier reflection of a quasiparticle from the defect potential. In this case, the velocity at which BP ‘falls’ on the barrier may be determined by a pulse of magnetic field applied to the BP. And, as we shall see bellow, the potential of interaction between the BP and a defect has a rather simple form. Obviously, the effect is more noticeable in the case when the BP energy is not much greater than the height of the potential barrier *U*_{0}.

*H*

_{ y }(

*t*) =

*H*

_{0}

*χ*(1 −

*t*/

*T*) in the form

where *v* = ∂*z*_{0}/∂*t* is the BP velocity, *χ*(1 − *t*/*T*) is the Heaviside function, *H*_{0} is the amplitude, and *T* is the pulse duration.

*v*(

*t*) =

*π*

^{2}

*M*

_{ S }ΛΔ

*H*

_{0}

*T*/

*m*

_{BP}. Accordingly, the energy of the BP in current time range

*E*

_{BP}is given by

Note that the study, performed for time $\mathit{t}<<{\mathit{\alpha}}^{-1}{\mathit{\omega}}_{\mathit{M}}^{-1}$ (or with taking into account the value of the magnetization decay *ω*_{
M
}*t* < < 10^{2} − 10^{3}), allows us to neglect the effect on the process of the braking force $\tilde{\mathit{F}}~\mathit{\alpha}{\mathit{\omega}}_{\mathit{M}}{\mathit{m}}_{\mathrm{\text{BP}}}\mathit{v}.$

*z*

_{0}= 0. Then, by expanding the potential of interaction of BP with the defect,

*U*

_{ d }(

*z*

_{0}), in a series near this point and taking Equation 2 into account, we can write down

where in accordance with the formula (2), the height of the potential barrier is *U*_{0} = *π*^{2}Λ^{2}Δ*M*_{
S
}*H*_{
c
}.

Note that phenomenological expression for defect-effective field *H*_{
d
} (see formula (4)) follows from the series expansion of the potential *U*_{
d
}(*z*_{0}) near the inflection point. It was at this point that there is maximum field of defect. It is natural to assume that if BP has overcome the barrier in this point, then the tunneling process is probable in general.

*R*by the formula

where $\mathit{\beta}=-\frac{2}{\mathit{\hslash}}\mathrm{Im}{\displaystyle \underset{{\mathit{z}}_{0,1}^{\ast}}{\overset{{\mathit{z}}_{0,2}^{\ast}}{\int}}\mathit{dz}\sqrt{2{\mathit{m}}_{\mathrm{\text{BP}}}\left({\mathit{E}}_{\mathrm{\text{BP}}}-{\mathit{U}}_{\mathit{d}}\left(\mathit{z}\right)\right)}}$${\mathit{z}}_{0,2}^{\ast}$, and ${\mathit{z}}_{0,2}^{\ast}$ are the roots of the equation *E*_{BP} − *U*_{
d
}(*z*_{0}) = 0.

where the parameter *ϵ*′ = (*E*_{BP} − *U*_{0})/*E*_{BP} < < 1 (recall that we consider the case when the energy *E*_{BP} close to *U*_{0}).

Substituting into the expressions (15) and (17), the ferromagnet and defect parameters, at *ϵ*′ ≥ 5 × 10^{−5} we obtain *R* ≤ 0.1, which is in accordance with criterion of applicability of Equation 15 (see [28]).

Note that from Equations 15 and 16, it follows that *R* → 0 at *U*_{0} → 0, i.e., we obtain a physically consistent conclusion about the disappearance of the effect of over-barrier reflection in the absence of a potential barrier.

Based on the obvious relation, $\mathit{\tau}~\mathrm{\Delta}{\left(\frac{{\mathit{m}}_{\mathrm{\text{BP}}}}{{\mathit{U}}_{0}}\right)}^{1/2}=\frac{4}{{\mathit{\omega}}_{\mathit{M}}}{\left(\frac{{\mathit{M}}_{\mathit{S}}}{{\mathit{H}}_{\mathit{c}}}\right)}^{1/2}{\mathit{Q}}^{-1/2}$ and the numerical data, given above, we determine *τ*, the characteristic time of interaction of BP with the defect 0.6 ≤ *ω*_{
M
}*τ* ≤ 2.3. It is easy to see that *τ* satisfies the relation *ω*_{
M
}*τ* < *ω*_{
M
}*t* ~ 10 − 10^{2}, which together with an estimate for *R* indicates on the possibility of the quantum phenomenon under study. In this case, the analysis of expressions (13) and (14) shows that the amplitude of a pulsed magnetic field is *H*_{0} ~ 4*π*(*M*_{
S
}*H*_{
c
})^{1/2}/*ω*_{
M
}*T* < 8*M*_{
S
}, which is consistent with the requirement for values of the planar magnetic fields applied to DW in ferromagnets [1].

*E*

_{BP}≈

*U*

_{0}, then the conditions of ‘quasi-classical’ behavior of the Bloch point and the potential barrier actually coincide and, in accordance with [24], are reduced to the fulfillment of the inequality

where $\mathit{\delta}{\mathit{z}}_{0}=\mathrm{\Delta}\sqrt{2\left({\mathit{E}}_{\mathrm{\text{BP}}}-{\mathit{U}}_{0}\right)/{\mathit{U}}_{0}}\approx \mathrm{\Delta}\sqrt{2{\mathit{\u03f5}}^{\prime}}.$

*U*

_{0}, Equation 18 can be rewritten as

*ϵ*′ ≥ 10

^{−4}, that in fact is a ‘lower estimate’ for this parameter. In a critical temperature ${\mathit{T}}_{\mathit{c}}^{*}$, corresponding to the given effect, we determine from the exponent in the formula (15) using the relation ${\mathit{k}}_{\mathit{B}}{\mathit{T}}_{\mathit{c}}^{\ast}={\mathit{\beta}}^{-1}\left({\mathit{E}}_{\mathrm{\text{BP}}}-{\mathit{U}}_{0}\right)$. Then, taking into account Equation 17, finally, we get

An estimate of the expression (19) shows that ${\mathit{T}}_{\mathit{c}}^{\ast}~\left({10}^{-3}-{10}^{-2}\right)$ K. Such values of ${\mathit{T}}_{\mathit{c}}^{\ast}$ are in the same range with critical temperatures for processes of quantum tunneling of DW [13], vertical BL [14] and BP through a defect. This fact indicates the importance of considering the effect of over-barrier reflection of BP in the study of quantum properties of these magnetic inhomogeneities.

## Conclusions

It is shown that in the subhelium temperature range, the Bloch point manifest themselves as a quantum mechanical object. Thus, the BP may tunnel through the pining barrier formed by the defect and over-barrier reflection from the defect potential. In this case, since the over-barrier reflection of the BP and sub-barrier tunneling of the BP occur in pulse and permanent magnetic fields, respectively, the practical possibility to study these quantum phenomena separately exists. Moreover, the experimental realization of the mentioned phenomena can be the basis for the creation of new methods of diagnostic of ferromagnetic materials and sensitive methods for studying an internal structure of their DWs.

## Declarations

## Authors’ Affiliations

## References

- Malozemoff AP, Slonczewski JC:
*Magnetic Domain Walls in Bubble Materials*. New York: Academic Press; 1979.Google Scholar - Konishi A: A new-ultra-density solid state memory: Bloch line memory.
*IEEE Trans. Magn.*1838, 1983: 19.Google Scholar - Klaui M, Vaz CAF, Bland JAC: Head-to-head domain-wall phase diagram in mesoscopic ring magnets.
*Appl. Phys. Lett.*2004, 85: 5637. 10.1063/1.1829800View ArticleGoogle Scholar - Laufenberg M, Backes D, Buhrer W: Observation of thermally activated domain wall transformations.
*Appl. Phys. Lett.*2006, 88: 052507. 10.1063/1.2168677View ArticleGoogle Scholar - Nakatani Y, Thiaville A, Miltat J: Head-to-head domain walls in soft nano-strips: a refined phase diagram.
*JMMM*2005, 290–291: 750.View ArticleGoogle Scholar - Vukadinovic N, Boust F: Three-dimensional micromagnetic simulations of multidomain bubble-state excitation spectrum in ferromagnetic cylindrical nanodots.
*Phys. Rev. B*2008, 78: 184411.View ArticleGoogle Scholar - Takagi S, Tatara G: Macroscopic quantum coherence of chirality of a domain wall in ferromagnets.
*Phys. Rev. B*1996, 54: 9920. 10.1103/PhysRevB.54.9920View ArticleGoogle Scholar - Shibata J, Takagi S: Macroscopic quantum dynamics of a free domain wall in a ferromagnet.
*Phys. Rev. B*2000, 62: 5719. 10.1103/PhysRevB.62.5719View ArticleGoogle Scholar - Galkina EG, Ivanov BA, Savel’ev S: Chirality tunneling and quantum dynamics for domain walls in mesoscopic ferromagnets.
*Phys. Rev. B*2009, 77: 134425.View ArticleGoogle Scholar - Ivanov BA, Kolezhuk AK: Quantum tunneling of magnetization in a small area – domain wall.
*JETP Letters*1994, 60: 805.Google Scholar - Ivanov BA, Kolezhuk AK, Kireev VE: Chirality tunneling in mesoscopic antiferromagnetic domain walls.
*Phys. Rev. B*1999, 58: 11514.View ArticleGoogle Scholar - Dobrovitski VV, Zvezdin AK: Macroscopic quantum tunnelling of solitons in ultrathin films.
*JMMM*1996, 156: 205. 10.1016/0304-8853(95)00756-3View ArticleGoogle Scholar - Chudnovsky EM, Iglesias O, Stamp PCE: Quantum tunneling of domain walls in ferromagnets.
*Phys. Rev. B*1992, 46: 5392. 10.1103/PhysRevB.46.5392View ArticleGoogle Scholar - Shevchenko AB: Quantum tunneling of a Bloch line in the domain wall of a cylindrical magnetic domain.
*Techn. Phys.*2007, 52: 1376. 10.1134/S1063784207100222View ArticleGoogle Scholar - Dobrovitski VV, Zvezdin AK: Quantum tunneling of a domain wall in a weak ferromagnet.
*JETP*1996, 82: 766.Google Scholar - Lisovskii VF:
*Fizika tsilindricheskikh magnitnykh domenov (Physics of Magnetic Bubbles)*. Moscow: Sov. Radio; 1982.Google Scholar - Thiaville A, Garcia JM, Dittrich R: Micromagnetic study of Bloch-point-mediated vortex core reversal.
*Phys. Rev. B*2003, 67: 094410.View ArticleGoogle Scholar - Kufaev YA, Sonin EB: Dynamics of a Bloch point (point soliton) in a ferromagnet.
*JETP*1989, 68: 879.Google Scholar - Zubov VE, Krinchik GS, Kuzmenko SN: Anomalous coercive force of Bloch point in iron single crystals.
*JETP Lett*1990, 51: 477.Google Scholar - Kabanov YP, Dedukh LM, Nikitenko VI: Bloch points in an oscillating Bloch line.
*JETP Lett*1989, 49: 637.Google Scholar - Gornakov VS, Nikitenko VI, Prudnikov IA: Mobility of the Bloch point along the Bloch line.
*JETP Lett*1989, 50: 513.Google Scholar - Chudnovsky EM: Macroscopic quantum tunneling of the magnetic moment.
*J. Appl. Phys.*1993, 73: 6697. 10.1063/1.352507View ArticleGoogle Scholar - Vaninstein AI, Zakharov VI, Novikov VA, Shifman MA: ABS of instantons.
*Sov. Phys. Usp*1982, 25: 195.View ArticleGoogle Scholar - Landau LD, Lifshitz EM:
*Kvantovaya mekhanika (Quantum Mechanics)*. Moscow: Nauka; 1989.Google Scholar - Galkina EG, Ivanov BA, Stephanovich VA: Phenomenological theory of Bloch point relaxation.
*JMMM*1993, 118: 373. 10.1016/0304-8853(93)90441-4View ArticleGoogle Scholar - Bar’yakhtar VG: Phenomenological description of relaxation processes in magnetic materials.
*JETP*1984, 60: 863.Google Scholar - Pokrovskii VL, Khalatnikov EM: К voprosu о nadbarjernom otrazhenii chastiz visokih energiy (On supperbarrier reflection of high energy particles).
*Eksp Z Teor. Fiz.*1961, 40: 1713.Google Scholar - Elyutin PV, Krivchenkov VD:
*Kvantovaya mekhanika (Quantum Mechanics)*. Moscow: Nauka; 1976.Google Scholar

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